Exchange-Striction Driven Ultrafast Nonthermal Lattice Dynamics in NiO

نویسندگان

چکیده

We use femtosecond electron diffraction to study ultrafast lattice dynamics in the highly correlated antiferromagnetic (AFM) semiconductor NiO. Using scattering vector ($Q$) dependence of Bragg diffraction, we introduce $Q$-resolved effective temperatures describing transient lattice. identify a nonthermal state with preferential displacement O compared Ni ions, which occurs within $\ensuremath{\sim}0.3\text{ }\text{ }\mathrm{ps}$ and persists for 25 ps. associate this changes AFM exchange striction-induced distortion, supported by observation $Q$ asymmetry Friedel pairs. Our highlights role spin-lattice coupling routes towards control spin order.

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ژورنال

عنوان ژورنال: Physical Review Letters

سال: 2021

ISSN: ['1079-7114', '0031-9007', '1092-0145']

DOI: https://doi.org/10.1103/physrevlett.126.147202